Publications

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[63] Marreiros, J., Van Dommelen, L., de Oliveira-Silva, R., Fleury, G., Iacomi, P., Stassin, T., Furukawa, S., Llewellyn, P., Sakellariou, D., Roeffaers, R., and Ameloot, R., Vapor‐phase linker exchange of the metal‐organic framework ZIF‐8: a solvent‐free approach to post‐synthetic modification. Angewandte Chemie International Edition (2019). Link to Publisher PDF

 

[62] Iacomi, P., Formalik, F., Marreiros, J., Shang J., Rogacka, J., Mohmeyer, A., Behrens, P., Ameloot, R., Kuchta, B., and Llewellyn, P. L., Role of structural defects in the adsorption and separation of C3 hydrocarbons in Zr-fumarate-MOF (MOF-801). Chemistry of Materials (2019). Link to Publisher PDF

 

[61] Krishtab, M., Stassen, I., Stassin, T., Cruz, A. J., Okudur, O. O., Armini, S., Wilson, C., De Gendt, S., and Ameloot, R., Vapor-deposited zeolitic imidazolate frameworks as gap-filling ultra-low-k dielectrics. Nature Communications 10, 3729 (2019). Link to Publisher PDF

Highlighted in Nature Communications (Editor's Highlights, August 2019), imec, KU Leuven news, eeNews, Phys.org, Electronics Weekly, Nanowerk News, Leuven Mindgate, Engineers Online, Science Daily, Electronics Specifier, New Electronics

 

[60] Stassin, T., Rodríguez-Hermida, S., Schrode, B., Cruz, A. J., Carraro, F., Kravchenko, D., Creemers, V., Stassen, I., Hauffman, T., De Vos, D. E., Falcaro, P., Resel R., and Ameloot, R., Vapour-phase deposition of oriented copper dicarboxylate metal–organic framework thin films. Chemical Communications, 55, 10056 - 10059 (2019). Link to Publisher PDF

Front Cover of ChemComm Issue 68, September 2019

 

[59] Piovesan, A., Achille, C., Ameloot, R., Nicolai, B., and Verboen, P., Pore network model for permeability characterization of 3D printed porous materials for passive microfluidics. Physical Review E 99, 033107 (2019). Link to Publisher PDF


[58] Marreiros, J., Caratelli, C., Hajek, J., Krajnc, A., Fleury, G., Bueken, B., De Vos, D., Mali, G., Roeffaers, M., Van Speybroeck, V., and Ameloot, R., The active role of methanol in post-synthetic linker exchange in the metal-organic framework UiO-66. Chemistry of Materials 31 (4), 1359–1369 (2019). Link to Publisher PDF

 

[57] Tu, M., Reinsch, H., Rodríguez-Hermida, S., Verbeke, R., Stassin, T., Egger, W., Dickmann, M., Dieu, Bjorn., Hofkens, J., Vankelecom, I., Stock, N., and Ameloot, R., Reversible Optical Writing and Data Storage in an Anthracene-Loaded Metal-Organic Framework. Angewandte Chemie-International Edition 58, 2423-2427 (2019). Link to Publisher PDF

 

[56] Saouma, C. T., Tsou, C., Richard, S., Ameloot, R., Vermoortele, F., Smolders, S., Bueken, B., DiPasquale, A. G., Kaminsky, W., Valdeza, C.N., De Vos, D. E., and Mayer, J.M., Sodium-coupled electron transfer reactivity of metal-organic frameworks containing titanium clusters: the importance of cations in redox chemistry. Chemical Science 10, 1322-1331(2018). Link to Publisher PDF

 

[55] Saouma, C.T., Richard, S., Smolders, S., Delley, M., Ameloot, R., Vermoortele, F., De Vos, D. E., and Mayer, J., Bulk-to-Surface Proton-Coupled Electron Transfer Reactivity of the Metal-Organic Framework MIL-125. Journal of the American Chemical Society 140 (47), 16184–16189 (2018). Link to Publisher PDF

 

[54] Wuttke, S., Medina, D. D., Rotter, J.M., Begum, S., Stassin, T., Ameloot, R., Oschatz, M., and Tsotsalas, M., Bringing Porous Organic and Carbon-Based Materials toward Thin-Film Applications. Advanced Functional Materials 28, 1801545 (2018). Link to Publisher PDF

 

[53] Parra-Cabrera, C., Achille, C., Kuhn, S., and Ameloot, R., 3D printing in chemical engineering and catalytic technology: structured catalysts, mixers, and reactors. Chemical Society Reviews 47, 209-230 (2018). Link to Publisher PDF

 

[52] Verduyckt, J., Geers, A., Claes, B., Eyley, S., Van Goethem, C., Stassen, I., Smolders, S., Ameloot, R., Vankelecom, I., Thielemans, W., and De Vos, D. E., Stabilising Ni catalysts for the dehydration–decarboxylation–hydrogenation of citric acid to methylsuccinic acid. Green Chemistr19, 4642-4650 (2017). Link to Publisher PDF

 

[51] Stassen, I., Boldog, I., Steuwe, C., De Vos, D. E., Roeffaers, M., Furukawa, S., and Ameloot, R., Photopatterning of fluorescent host-guest carriers through pore activation of metal-organic framework single crystals. Chemical Communications 53, 7222-7225 (2017). Link to Publisher PDF

Outside Front Cover ChemComm Emerging Investigators 2017

 

[50] Stassen, I., Burtch, N., Talin, A., Falcaro, P., Allendorf, M., and Ameloot, R., An updated roadmap for the integration of metal-organic frameworks with electronic devices and chemical sensors. Chemical Society Reviews 46, 3185-3241 (2017). Link to Publisher PDF

Back Cover ChemSocRev 2017 

 

[49] Vandezande, W., Janssen, K., Delport, F., Ameloot, R., De Vos, D. E., Lammertyn, J., and Roeffaers, M., Parts per million detection of alcohol vapors via metal-organic framework functionalized surface plasmon resonance sensors. Analytical Chemistry 89 (8), 4480–4487 (2017). Link to Publisher PDF

 

[48] Bueken, B., Van Velthoven, N., Willhammar, T., Stassin, T., Stassen, I., A. Keen, D., Ameloot, R., Bals, S., De Vos, D. E., and Bennett, T., Gel-Based Morphological Design of Zirconium Metal-organic Frameworks. Chemical Science 8, 3939–3948 (2017). Link to Publisher PDF

 

[47] Bueken, B., Reinsch H., Heidenreich, N., Vandekerkhove, A., Vermoortele, F., Kirschhock, C. E. A., Stock, N., De Vos, D. E., and Ameloot, R., Investigation of the water-induced phase transformation of UTSA-74 to MOF-74(Zn). CrystEngCom 19, 4152-4156 (2017). Link to Publisher PDF

 

[46] Stassin, T., Reinsch, H., Van de Voorde, B., Wuttke, S., D. Medina, D., Stock, N., Bein, T., Ameloot, R., and De Vos, D. E., Adsorption and Reactive Desorption on Metal-Organic Frameworks: A Direct Strategy for Lactic Acid Recovery. ChemSusChem 10 (3), 643–650 (2017). Link to Publisher PDF

 

[45] Stassen, I., De Vos, D. E., and Ameloot, R., Vapor-Phase Deposition and Modification of Metal-Organic Frameworks: State-of-the-Art and Future Directions. Chemistry - A European Journal 22 (41), 14452–14460 (2016). Link to Publisher PDF

 

[44] Deleu, W.P.R, Stassen, I., Jonckheere, D., Ameloot, R., De Vos, D. E. Waste PET (bottles) as Resource or Substrate for MOF Synthesis. Journal of Materials Chemistry A 4, 9519-9525 (2016). Link to Publisher PDF

 

[43] Stassen, I., Bueken, B., Reinsch, H., Oudenhoven, J.F.M., Wouters, D., Hajek, J., Van Speybroeck, V., Stock,N., Vereecken,P.M. , Van Schaijk,R., De Vos, D. E., and Ameloot, R., Towards Metal-Organic Framework based Field Effect Chemical Sensors: UiO-66-NH2 for Nerve Agent Detection. Chemical Science 7, 5827-5832 (2016). Link to Publisher PDF

Highlighted in Reuters, BBC show The Naked Scientists, National Geographic, FOX News, Knack, EOS Wetenschap, ErekAlert!, Nanowerk, Nature World News, ChemInfo
More highlights here

 

[42] Hulsbosch, J., De Vos, D. E., Binnemans, K., and Ameloot, R., Bio-based ionic liquids: solvents for a green processing industry. ACS Sustainable Chemistry and Engineering. 4 (6), 2917–2931 (2016). Link to Publisher PDF

 

[41] Jonckheere, D., Coutino-Gonzalez, E., Baekelant, W., Bueken, B, Reinsch, H., Stassen, I., Fenwick, O., Richard, F., Samorì, P., Ameloot, R., Hofkens, J., Roeffaers, M., and De Vos, D. E., Silver-induced reconstruction of an adeninate-based metal-organic framework for encapsulation of luminescent adenine-stabilized silver clusters. Journal of Materials Chemistry C 4, 4259-4268 (2016). Link to Publisher PDF

 

[40] Lohse, M. S., Stassin, T., Naudin, G., Wuttke, S., Ameloot, R., De Vos, D. E., Medina, D. D., and Bein, T., Sequential Pore Wall Modification in a Covalent Organic Framework for Application in Lactic Acid Adsorption. Chemistry of Materials 28, 626–631 (2016). Link to Publisher PDF

 

[39] Stassen, I., Styles, M., Grenci, G., Gorp, H. V., Vanderlinden, W., Feyter, S. D., Falcaro, P., DeVos, D. E., Vereecken, P., and Ameloot, R., Chemical vapour deposition of zeolitic imidazolate framework thin films. Nature Materials 15304–310 (2016). Link to Publisher PDF

Front Cover Nature Materials March 2016
Highlighted in Nature Materials. Allendorf, M. D., and Stavila, V., Nanoporous films: From conventional to conformal.
Further highlights: KnackEurekAlert!Phys.orgNanowerkScience DailyMaterials TodayMaterials Today (2)Asian Scientist MagazineTechnology.orgChemInfoBioportfolio

 

[38] Falcaro, P., Ricco, R., Yazdi, A., Imaz, I., Furukawa, S., Maspoch, D., Ameloot, R., Evans, J. D., and Doonan, C. J., Application of metal and metal oxide nanoparticles@MOFs. Coordination Chemistry Reviews 307, Part 2, 237–254 (2015). Link to Publisher PDF

 

[37] Valvekens, P., Bloch, E. D., Long, J. R., Ameloot, R., and De Vos, D. E. Counteranion effects on the catalytic activity of copper salts immobilized on the 2,2′-bipyridine-functionalized metal-organic framework MOF-253. Catalysis Today 246, 55–59 (2015). Link to Publisher PDF

 

[36] Stassen, I., Styles, M., Van Assche, T., Campagnol, N., Fransaer, J., Denayer, J., Tan, J.-C., Falcaro, P., De Vos, D. E., and Ameloot, R., Electrochemical Film Deposition of the Zirconium Metal-Organic Framework UiO-66 and Application in a Miniaturized Sorbent Trap. Chemistry of Materials 27, 1801-1807 (2015). Link to Publisher PDF

 

[35] Humbeck, J. F. V., Aubrey, M. L., Alsbaiee, A., Ameloot, R., Coates, G. W., Dichtel, W. R. and Long, J. R., Tetraarylborate polymer networks as single-ion conducting solid electrolytes. Chemical Science 6, 5499–5505 (2015). Link to Publisher PDF

 

[34] Glas, D., Paesen, R., Depuydt, D., Binnemans, K., Ameloot, M., De Vos, D. E., and Ameloot, R., Cellulose amorphization by swelling in ionic liquid/water mixtures: a combined macroscopic and second-harmonic microscopy study. ChemSusChem 8, 82–86 (2015). Link to Publisher PDF

 

[33] Bueken, B., Vermoortele, F., Vanpoucke, D. E. P., Reinsch, H., Tsou, C.-C., Valvekens, P., De Baerdemaeker, T., Ameloot, R., Kirschhock, C. E. A., Van Speybroeck, V., Mayer, J. M., and De Vos, D. E., A Flexible Photoactive Titanium Metal-Organic Framework Based on a [TiIV3(μ3-O)(O)2(COO)6] Cluster. Angewandte Chemie International Edition 54, 13912–13917 (2015). Link to Publisher PDF

 

[32] Voorde, B. V. de, Stassen, I., Bueken, B., Vermoortele, F., Vos, D. D., Ameloot, R., Tan, J.-C., and Bennett, T. D., Improving the mechanical stability of zirconium-based metal-organic frameworks by incorporation of acidic modulators. Journal of Materials Chemistry A 3, 1737–1742 (2014). Link to Publisher PDF

 

[31] Reinsch, H., Stassen, I., Bueken, B., Lieb, A., Ameloot, R., and De Vos D. E., First examples of aliphatic zirconium MOFs and the influence of inorganic anions on their crystal structures. CrystEngComm 17, 331–337 (2014). Link to Publisher PDF

 

[30] Keitz, B. K., Yu, C. J., Long, J. R., and Ameloot, R., Lithographic Deposition of Patterned Metal-Organic Framework Coatings Using a Photobase Generator. Angewandte Chemie-International Edition 53, 5561–5565 (2014). Link to Publisher PDF

Highlighted in Nature Chemistry. Hansell, C.: Patterning with a light touch

 

[29] Bueken, B., Reinsch, H., Reimer, N., Stassen, I., Vermoortele, F., Ameloot, R., Stock, N., Kirschhock, C. E. A., and Vos, De Vos D. E., A zirconium squarate metal-organic framework with modulator-dependent molecular sieving properties. Chemical Communications 50, 10055–10058 (2014). Link to Publisher PDF

 

[28] Aubrey, M. L., Ameloot, R., Wiers, B. M., and Long, J. R., Metal-organic frameworks as solid magnesium electrolytes. Energy and Environmental Science 7, 667 (2014). Link to Publisher PDF

 

[27] Witters, D., Vermeir, S., Puers, R., Sels, B. F., De Vos, D. E., Lammertyn, J., and Ameloot, R., Miniaturized Layer-by-Layer Deposition of Metal-Organic Framework Coatings through Digital Microfluidics. Chemistry of Materials 25, 1021–1023 (2013). Link to Publisher PDF

 

[26] Van de Voorde, B., Ameloot, R., Stassen, I., Everaert, M., De Vos, D. E., and Tan, J.-C., Mechanical properties of electrochemically synthesised metal-organic framework thin films. Journal of Materials Chemistry C 1, 7716 (2013). Link to Publisher PDF

 

[25] Stassen, I., Campagnol, N., Fransaer, J., Vereecken, P., De Vos, D. E., and Ameloot, R., Solvent-free synthesis of supported ZIF-8 films and patterns through transformation of deposited zinc oxide precursors. CrystEngComm 15, 9308 (2013). Link to Publisher PDF

 

[24] Peeters, A., Valvekens, P., Ameloot, R., Sankar, G., Kirschhock, C. E. A., and De Vos, D. E., Zn–Co Double Metal Cyanides as Heterogeneous Catalysts for Hydroamination: A Structure-Activity Relationship. ACS Catalysis 3, 597–607 (2013). Link to Publisher PDF

 

[23] Peeters, A., Ameloot, R., and De Vos, D. E., Carbon dioxide as a reversible amine-protecting agent in selective Michael additions and acylations. Green Chemistry 15, 1550–1557 (2013). Link to Publisher PDF

 

[22] Laurier, K. G. M., Vermoortele, F., Ameloot, R., De Vos, D. E., Hofkens, J., and Roeffaers, M. B. J., Iron(III)-Based Metal-Organic Frameworks As Visible Light Photocatalysts. Journal of the American Chemical Society 135, 14488–14491 (2013).Link to Publisher PDF

 

[21] Ameloot, R., Vermoortele, F., Hofkens, J., De Schryver, F. C., De Vos, D. E., and Roeffaers, M. B. J., Three-Dimensional Visualization of Defects Formed during the Synthesis of Metal-Organic Frameworks: A Fluorescence Microscopy Study. Angewandte Chemie-International Edition 52, 401–405 (2013). Link to Publisher PDF

Highlighted in Nature. Serre, C.: Defects visualized in porous solids

 

[20] Ameloot, R., Aubrey, M., Wiers, B. M., Gómora-Figueroa, A. P., Patel, S. N., Balsara, N. P., and Long, J. R., Ionic Conductivity in the Metal-Organic Framework UiO-66 by Dehydration and Insertion of Lithium tert-Butoxide. Chemistry – A European Journal 19, 5533–5536 (2013). Link to Publisher PDF

 

[19] Witters, D., Vergauwe, N., Ameloot, R., Vermeir, S., De Vos, D. E, Puers, R., Sels, B., and Lammertyn, J., Digital Microfluidic High-Throughput Printing of Single Metal-Organic Framework Crystals. Advanced Materials 24, 1316–1320 (2012). Link to Publisher PDF

Highlighted in Nature Materials. Dusastre, V.: Printed MOFs

 

[18] Vermoortele, F., Vandichel, M., Van de Voorde, B., Ameloot, R., Waroquier, M., Van Speybroeck, V., and De Vos, D. E., Electronic Effects of Linker Substitution on Lewis Acid Catalysis with Metal-Organic Frameworks. Angewandte Chemie-International Edition 51, 4887–4890 (2012). Link to Publisher PDF

 

[17] Vermoortele, F., Ameloot, R., Alaerts, L., Matthessen, R., Carlier, B., Fernandez, E. V. R., Gascon, J., Kapteijn, F., and De Vos, D. E., Tuning the catalytic performance of metal-organic frameworks in fine chemistry by active site engineering. Journal of Materials Chemistry 22, 10313–10321 (2012). Link to Publisher PDF

 

[16] Van Assche, T. R. C., Desmet, G., Ameloot, R., De Vos, D. E., Terryn, H., and Denayer, J. F. M., Electrochemical synthesis of thin HKUST-1 layers on copper mesh. Microporous and Mesoporous Materials 158, 209–213 (2012). Link to Publisher PDF

 

[15] Sachse, A., Ameloot, R., Coq, B., Fajula, F., Coasne, B., De Vos, D. E., and Galarneau, A., In situ synthesis of Cu-BTC (HKUST-1) in macro-/mesoporous silica monoliths for continuous flow catalysis. Chemical Communications 48, 4749–4751 (2012). Link to Publisher PDF

 

[14] Maes, M., Vermoortele, F., Boulhout, M., Boudewijns, T., Kirschhock, C. E. A., Ameloot, R., Beurroies, I., Denoyel, R., and De Vos, D. E., Enthalpic effects in the adsorption of alkylaromatics on the metal-organic frameworks MIL-47 and MIL-53. Microporous and Mesoporous Materials 157, 82–88 (2012). Link to Publisher PDF

 

[13] Vermoortele, F., Ameloot, R., Vimont, A., Serre, C., and De Vos D. E., An amino-modified Zr-terephthalate metal-organic framework as an acid-base catalyst for cross-aldol condensation. Chemical Communications 47, 1521–1523 (2011). Link to Publisher PDF

 

[12] Peeters, A., Valvekens, P., Vermoortele, F., Ameloot, R., Kirschhock, C. E. A., and De Vos D. E., Lewis acid double metal cyanide catalysts for hydroamination of phenylacetylene. Chemical Communications 47, 4114–4116 (2011). Link to Publisher PDF

 

[11] Ameloot, R., Vermoortele, F., Vanhove, W., Roeffaers, M. B. J., Sels, B. F., and De Vos D. E., Interfacial synthesis of hollow metal-organic framework capsules demonstrating selective permeability. Nature Chemistry 3, 382–387 (2011). Link to Publisher PDF

Highlighted n Nature Materials. Russell E. M.: Metal-organic frameworks: Grown into shape

 

[10] Ameloot, R., Roeffaers, M. B. J., De Cremer, G., Vermoortele, F., Hofkens, J., Sels, B. F., and De Vos, D. E., Metal-Organic Framework Single Crystals as Photoactive Matrices for the Generation of Metallic Microstructures. Advanced Materials 23, 1788–1791 (2011). Link to Publisher PDF

 

[9] Maes, M., Alaerts, L., Vermoortele, F., Ameloot, R., Couck, S., Finsy, V., Denayer, J. F. M., and De Vos, D. E., Separation of C-5-Hydrocarbons on Microporous Materials: Complementary Performance of MOFs and Zeolites. Journal of the American Chemical Society 132, 2284–2292 (2010). Link to Publisher PDF

 

[8] Ameloot, R., Pandey, L., Van der Auweraer, M., Alaerts, L., Sels, B. F., and De Vos, D. E., Patterned film growth of metal-organic frameworks based on galvanic displacement. Chemical Communications 46, 3735–3737 (2010). Link to Publisher PDF

 

[7] Ameloot, R., Liekens, A., Alaerts, L., Maes, M., Galarneau, A., Coq, B., Desmet, G., Sels, B. F., Denayer, J. F. M., and De Vos, D. E., Silica-MOF Composites as a Stationary Phase in Liquid Chromatography. European Journal of Inorganic Chemistry 3735–3738 (2010). Link to Publisher PDF

Shared front cover

 

[6] Ameloot, R., Gobechiya, E., Uji-i, H., Martens, J. A., Hofkens, J., Alaerts, L., Sels, B. F., and De Vos, D. E., Direct Patterning of Oriented Metal-Organic Framework Crystals via Control over Crystallization Kinetics in Clear Precursor Solutions. Advanced Materials 22, 2685–2688 (2010). Link to Publisher PDF

 

[5] Roeffaers, M. B. J., De Cremer, G., Libeert, J., Ameloot, R., Dedecker, P., Bons, A. J., Buckins, M., Martens, J. A., Sels, B. F., De Vos, D. E., and Hofkens, J., Super-Resolution Reactivity Mapping of Nanostructured Catalyst Particles. Angewandte Chemie-International Edition 48, 9285–9289 (2009). Link to Publisher PDF

 

[4] Ameloot, R., Stappers, L., Fransaer, J., Alaerts, L., Sels, B. F., and De Vos, D. E., Patterned Growth of Metal-Organic Framework Coatings by Electrochemical Synthesis. Chemistry of Materials 21, 2580–2582 (2009). Link to Publisher PDF

 

[3] Ameloot, R., Roeffaers, M., Baruah, M., De Cremer, G., Sels, B., De Vos, D. E, and Hofkens, J., Towards direct monitoring of discrete events in a catalytic cycle at the single molecule level. Photochemical & Photobiological Sciences 8, 453–456 (2009). Link to Publisher PDF

Front cover

 

[2] Roeffaers, M. B. J., Ameloot, R., Bons, A. J., Mortier, W., De Cremer, G., de Kloe, R., Hofkens, J., De Vos, D. E., and Sels, B. F., Relating pore structure to activity at the subcrystal level for ZSM-5: An electron backscattering diffraction and fluorescence microscopy study. Journal of the American Chemical Society 130, 13516–13517 (2008). Link to Publisher PDF

 

[1] Roeffaers, M. B. J., Ameloot, R., Baruah, M., Uji-i, H., Bulut, M., De Cremer, G., Muller, U., Jacobs, P. A., Hofkens, J., Sels, B. F. and De Vos, D. E., Morphology of large ZSM-5 crystals unraveled by fluorescence microscopy. Journal of the American Chemical Society 130, 5763–5772 (2008). Link to Publisher PDF

 

 

 

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